Carbon-based Catalysts: Synthesis and Applications

M. J. Lazaro; S. Ascaso; S. Perez-Rodriguez; J. Calderon; M.E. Galvez; M.J. Nieto; Rafael Moliner; A. Boyano; D. Sebastian; C. Alegre; Laura Calvillo; Veronica Celorrio

doi:10.1016/j.crci.2015.06.006

Carbon-based Catalysts: Synthesis and Applications

M. J. Lazaro
, S. Ascaso
, S. Perez-Rodriguez
, J. Calderon
, M.E. Galvez
, M.J. Nieto
, Rafael Moliner
, A. Boyano
, D. Sebastian
, C. Alegre
, Laura Calvillo
, Veronica Celorrio

School of Chemistry

Research output: Contribution to journal › Article (Academic Journal) › peer-review

59 Citations (Scopus)

602 Downloads (Pure)

Abstract

This paper summarizes the main results obtained by the Fuel Combustion Group in three applications: (1) carbon-based catalysts for the selective catalytic reduction (SCR) process of NO_x, (2) Pt and Pt–Ru catalysts for direct alcohol fuel cells, (3) carbon-supported catalysts for the electroreduction of CO₂. Concerning the first aspect, low-cost catalysts able to work at lower temperatures have been prepared and compared with commercial catalysts; for the second one, new catalysts for methanol and ethanol electrochemical oxidation exhibiting current densities that are double those of the commercial ones have been developed; as regards the third one, carbon-supported catalysts for the electroreduction of CO₂ based on Fe and Pd were synthesized and tested. Formic acid was obtained as the main product on all Fe/C electrodes.

Original language	English
Pages (from-to)	1229-1241
Number of pages	13
Journal	Comptes Rendus Chimie
Volume	18
Issue number	11
Early online date	27 Oct 2015
DOIs	https://doi.org/10.1016/j.crci.2015.06.006
Publication status	Published - Nov 2015

Keywords

Novel carbon materials
Carbon supported catalysts
NOx reduction
Direct alcohol fuel cells
Electroreduction of CO2

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This is the author accepted manuscript (AAM). The final published version (version of record) is available online via Elsevier at http://www.sciencedirect.com/science/article/pii/S1631074815001599. Please refer to any applicable terms of use of the publisher.
Accepted author manuscript, 343 KBLicence: CC BY-NC-ND
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This is the author accepted manuscript (AAM). The final published version (version of record) is available online via Elsevier at http://www.sciencedirect.com/science/article/pii/S1631074815001599. Please refer to any applicable terms of use of the publisher.
Accepted author manuscript, 649 KBLicence: CC BY-NC-ND

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title = "Carbon-based Catalysts: Synthesis and Applications",

abstract = "This paper summarizes the main results obtained by the Fuel Combustion Group in three applications: (1) carbon-based catalysts for the selective catalytic reduction (SCR) process of NOx, (2) Pt and Pt{\textendash}Ru catalysts for direct alcohol fuel cells, (3) carbon-supported catalysts for the electroreduction of CO2. Concerning the first aspect, low-cost catalysts able to work at lower temperatures have been prepared and compared with commercial catalysts; for the second one, new catalysts for methanol and ethanol electrochemical oxidation exhibiting current densities that are double those of the commercial ones have been developed; as regards the third one, carbon-supported catalysts for the electroreduction of CO2 based on Fe and Pd were synthesized and tested. Formic acid was obtained as the main product on all Fe/C electrodes.",

keywords = "Novel carbon materials, Carbon supported catalysts, NOx reduction, Direct alcohol fuel cells, Electroreduction of CO2",

author = "Lazaro, \{M. J.\} and S. Ascaso and S. Perez-Rodriguez and J. Calderon and M.E. Galvez and M.J. Nieto and Rafael Moliner and A. Boyano and D. Sebastian and C. Alegre and Laura Calvillo and Veronica Celorrio",

year = "2015",

month = nov,

doi = "10.1016/j.crci.2015.06.006",

language = "English",

volume = "18",

pages = "1229--1241",

journal = "Comptes Rendus Chimie",

issn = "1631-0748",

publisher = "Academie des sciences",

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}

TY - JOUR

T1 - Carbon-based Catalysts

T2 - Synthesis and Applications

AU - Lazaro, M. J.

AU - Ascaso, S.

AU - Perez-Rodriguez, S.

AU - Calderon, J.

AU - Galvez, M.E.

AU - Nieto, M.J.

AU - Moliner, Rafael

AU - Boyano, A.

AU - Sebastian, D.

AU - Alegre, C.

AU - Calvillo, Laura

AU - Celorrio, Veronica

PY - 2015/11

Y1 - 2015/11

N2 - This paper summarizes the main results obtained by the Fuel Combustion Group in three applications: (1) carbon-based catalysts for the selective catalytic reduction (SCR) process of NOx, (2) Pt and Pt–Ru catalysts for direct alcohol fuel cells, (3) carbon-supported catalysts for the electroreduction of CO2. Concerning the first aspect, low-cost catalysts able to work at lower temperatures have been prepared and compared with commercial catalysts; for the second one, new catalysts for methanol and ethanol electrochemical oxidation exhibiting current densities that are double those of the commercial ones have been developed; as regards the third one, carbon-supported catalysts for the electroreduction of CO2 based on Fe and Pd were synthesized and tested. Formic acid was obtained as the main product on all Fe/C electrodes.

AB - This paper summarizes the main results obtained by the Fuel Combustion Group in three applications: (1) carbon-based catalysts for the selective catalytic reduction (SCR) process of NOx, (2) Pt and Pt–Ru catalysts for direct alcohol fuel cells, (3) carbon-supported catalysts for the electroreduction of CO2. Concerning the first aspect, low-cost catalysts able to work at lower temperatures have been prepared and compared with commercial catalysts; for the second one, new catalysts for methanol and ethanol electrochemical oxidation exhibiting current densities that are double those of the commercial ones have been developed; as regards the third one, carbon-supported catalysts for the electroreduction of CO2 based on Fe and Pd were synthesized and tested. Formic acid was obtained as the main product on all Fe/C electrodes.

KW - Novel carbon materials

KW - Carbon supported catalysts

KW - NOx reduction

KW - Direct alcohol fuel cells

KW - Electroreduction of CO2

U2 - 10.1016/j.crci.2015.06.006

DO - 10.1016/j.crci.2015.06.006

M3 - Article (Academic Journal)

SN - 1631-0748

VL - 18

SP - 1229

EP - 1241

JO - Comptes Rendus Chimie

JF - Comptes Rendus Chimie

IS - 11

ER -

Carbon-based Catalysts: Synthesis and Applications

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