TY - JOUR
T1 - Detection of a pair density wave state in UTe2
AU - Gu, Qiangqiang
AU - Carroll, Joseph
AU - Wang, Shuqiu
AU - Ran, Sheng
AU - Broyles, Christopher
AU - Siddiquee, Hasan
AU - Butch, Nicholas
AU - Saha, Shanta
AU - Paglione, Johnpierre
AU - J. C. Séamus, Davis
AU - Liu, Xiaolong
N1 - Funding Information: Research at the University of Maryland was supported by the Department of Energy Award No. DE-SC-0019154 (sample characterization), the Gordon and Betty Moore Foundation’s EPiQS Initiative through grant no. GBMF9071 (materials synthesis), NIST and the Maryland Quantum Materials Center. Q.G., X.L., J.P.C. and J.C.S.D. acknowledge support from the Moore Foundation’s EPiQS Initiative through grant GBMF9457. J.C.S.D. acknowledges support from the Royal Society under award R64897. J.P.C. and J.C.S.D. acknowledge support from Science Foundation Ireland under award SFI 17/RP/5445. S.W. and J.C.S.D. acknowledge support from the European Research Council (ERC) under award DLV-788932.
PY - 2023/6/28
Y1 - 2023/6/28
N2 - Spin-triplet topological superconductors should exhibit many unprecedented electronic properties, including fractionalized electronic states relevant to quantum information processing. Although UTe2 may embody such bulk topological superconductivity, its superconductive order parameter Δ(k) remains unknown. Many diverse forms for Δ(k) are physically possible in such heavy fermion materials13. Moreover, intertwined density waves of spin (SDW), charge (CDW) and pair (PDW) may interpose, with the latter exhibiting spatially modulating superconductive order parameter Δ(r), electron-pair density and pairing energy gap. Hence, the newly discovered CDW state in UTe2 motivates the prospect that a PDW state may exist in this material. To search for it, we visualize the pairing energy gap with μeV-scale energy resolution using superconductive scanning tunnelling microscopy (STM) tips. We detect three PDWs, each with peak-to-peak gap modulations of around 10 μeV and at incommensurate wavevectors Pi=1,2,3 that are indistinguishable from the wavevectors Qi=1,2,3 of the prevenient CDW. Concurrent visualization of the UTe2 superconductive PDWs and the non-superconductive CDWs shows that every Pi:Qi pair exhibits a relative spatial phase δϕ ≈ π. From these observations, and given UTe2 as a spin-triplet superconductor, this PDW state should be a spin-triplet PDW. Although such states do exist in superfluid 3He, for superconductors, they are unprecedented.
AB - Spin-triplet topological superconductors should exhibit many unprecedented electronic properties, including fractionalized electronic states relevant to quantum information processing. Although UTe2 may embody such bulk topological superconductivity, its superconductive order parameter Δ(k) remains unknown. Many diverse forms for Δ(k) are physically possible in such heavy fermion materials13. Moreover, intertwined density waves of spin (SDW), charge (CDW) and pair (PDW) may interpose, with the latter exhibiting spatially modulating superconductive order parameter Δ(r), electron-pair density and pairing energy gap. Hence, the newly discovered CDW state in UTe2 motivates the prospect that a PDW state may exist in this material. To search for it, we visualize the pairing energy gap with μeV-scale energy resolution using superconductive scanning tunnelling microscopy (STM) tips. We detect three PDWs, each with peak-to-peak gap modulations of around 10 μeV and at incommensurate wavevectors Pi=1,2,3 that are indistinguishable from the wavevectors Qi=1,2,3 of the prevenient CDW. Concurrent visualization of the UTe2 superconductive PDWs and the non-superconductive CDWs shows that every Pi:Qi pair exhibits a relative spatial phase δϕ ≈ π. From these observations, and given UTe2 as a spin-triplet superconductor, this PDW state should be a spin-triplet PDW. Although such states do exist in superfluid 3He, for superconductors, they are unprecedented.
U2 - 10.1038/s41586-023-05919-7
DO - 10.1038/s41586-023-05919-7
M3 - Article (Academic Journal)
C2 - 37380691
SN - 0028-0836
VL - 618
SP - 921
EP - 927
JO - Nature
JF - Nature
ER -