Estimating source regions of European emissions of trace gases from observations at Mace Head

DB Ryall*, RG Derwent, AJ Manning, PG Simmonds, S O'Doherty

*Corresponding author for this work

Research output: Contribution to journalArticle (Academic Journal)peer-review

57 Citations (Scopus)

Abstract

A technique is described for identifying probable source locations for a range of greenhouse and ozone-depleting trace gases from the long-term measurements made at Mace Head, Ireland. The Met. Office's dispersion model NAME is used to predict concentrations at Mace Head from all possible sources in Europe, then source regions identified as those which consistently lead to elevated concentrations at Mace Head. Estimates of European emissions and their distribution are presented for a number of trace gases for the period 1995-1998. Estimated emission patterns are realistic, given the nature and varied applications of the species considered. The results indicate that whilst there are limitations, useful information about source distribution can be extracted from continuous measurements at a remote site. It is probable that much improved estimates could be derived if observations were available from a number of sites. The ability to assess emissions has obvious implications in monitoring compliance with internationally agreed quota and protocols. Crown Copyright (C) 2001 Published by Elsevier Science Ltd. All rights reserved.

Original languageEnglish
Pages (from-to)2507-2523
Number of pages17
JournalAtmospheric Environment
Volume35
Issue number14
Publication statusPublished - 2001

Keywords

  • Lagrangian dispersion model
  • inversion techniques
  • European emissions
  • greenhouse gases
  • ozone depleting gases
  • IRELAND
  • TRENDS

Cite this