Experimental determination of configurational entropy in a two-dimensional liquid under random pinning

Ian Williams, Francesco Turci, James E. Hallett, Peter Crowther, Chiara Cammarota, Giulio Biroli, C. Patrick Royall

Research output: Contribution to journalArticle (Academic Journal)peer-review

6 Citations (Scopus)
179 Downloads (Pure)

Abstract

A quasi two-dimensional colloidal suspension is studied under the influence of immobilisation (pinning) of a random fraction of its particles. We introduce a novel experimental method to perform random pinning and, with the support of numerical simulation, we find that increasing the pinning concentration smoothly arrests the system, with a cross-over from a regime of high mobility and high entropy to a regime of low mobility and low entropy. At the local level, we study fluctuations in area fraction and concentration of pins and map them to entropic structural signatures and local mobility, obtaining a measure for the local entropic fluctuations of the experimental system.

Original languageEnglish
Article number094003
Number of pages15
JournalJournal of Physics Condensed Matter
Volume30
Issue number9
Early online date12 Feb 2018
DOIs
Publication statusPublished - 7 Mar 2018

Keywords

  • entropy
  • glass transition
  • random pinning

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