Narrow and Stable Single Photon Emission from Dibenzoterrylene in para‐Terphenyl Nanocrystals

Ross C. Schofield*, Paul Burdekin, Anastasios Fasoulakis, Louise Devanz, Dominika P. Bogusz, Rowan A. Hoggarth, Kyle D. Major, Alex S. Clark*

*Corresponding author for this work

Research output: Contribution to journalArticle (Academic Journal)peer-review

9 Citations (Scopus)

Abstract

Single organic molecules are promising photon sources for quantum technologies. In this work we show photon emission from dibenzoterrylene, a widely used organic emitter, in a new host matrix, para-terphenyl. We present a reprecipitation growth method that produces para-terphenyl nanocrystals which are ideal for integration into nanophotonic devices due to their small size. We characterise the optical properties of dibenzoterrylene in nanocrystals at room and cryogenic temperatures, showing bright, narrow emission from a single molecule. Spectral data on the vibrational energies is presented and a further 25 additional molecules are characterised. This emitter-host combination has potential for quantum technology purposes with wavelengths suitable for interfacing with quantum memories.
Original languageEnglish
Article numbere202100809
Number of pages8
JournalChemPhysChem
Volume23
Issue number4
Early online date14 Dec 2021
DOIs
Publication statusPublished - 16 Feb 2022

Research Groups and Themes

  • QETLabs

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