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Novel experimental techniques and computational methods have provided new insight into the behavior of reactive intermediates in solution. The results of these studies show that some of the earlier ideas about how reactive intermediates ought to behave in solution were incomplete or even incorrect. This Perspective summarizes the new experimental and computational methods and draws attention to the shortcomings that their application has brought to light in previous models. Key areas needing further research are highlighted.
Original languageEnglish
Pages (from-to)4695-4705
Number of pages11
JournalJournal of the American Chemical Society
Issue number14
Early online date23 Mar 2016
Publication statusPublished - 13 Apr 2016


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