The transition from liquid to solid-like behaviour in ultrahigh viscosity aerosol particles

R. M. Power; S. H. Simpson; J. P. Reid; A. J. Hudson

doi:10.1039/c3sc50682g

The transition from liquid to solid-like behaviour in ultrahigh viscosity aerosol particles

R. M. Power
, S. H. Simpson
, J. P. Reid^*
, A. J. Hudson

^*Corresponding author for this work

Research output: Contribution to journal › Article (Academic Journal) › peer-review

188 Citations (Scopus)

Abstract

For the first time, a measurement of the viscosity of microparticles composed of Newtonian fluids has been made over a range of 12 orders of magnitude (10(-3) to 10(9) Pa s), extending from dilute aqueous solutions to the solid-like behaviour expected on approaching a glass transition. Using holographic optical tweezers to induce coalescence between two aerosol particles (volume

Original language	English
Pages (from-to)	2597-2604
Number of pages	8
Journal	Chemical Science
Volume	4
Issue number	6
DOIs	https://doi.org/10.1039/c3sc50682g
Publication status	Published - 1 Jun 2013

Research Groups and Themes

Physical & Theoretical

Keywords

HYGROSCOPICITY MODEL FRAMEWORK
SECONDARY ORGANIC AEROSOL
SUCROSE SOLUTIONS
GLASS-TRANSITION
SODIUM-CHLORIDE
PHASE-TRANSITIONS
AQUEOUS-SOLUTIONS
OPTICAL TWEEZERS
WATER
TEMPERATURE

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10.1039/c3sc50682g

http://pubs.rsc.org/en/Content/ArticleLanding/2013/SC/c3sc50682g#!divAbstract

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Cite this

@article{0aae2944a7eb4b7987e361cd714c0a8a,

title = "The transition from liquid to solid-like behaviour in ultrahigh viscosity aerosol particles",

abstract = "For the first time, a measurement of the viscosity of microparticles composed of Newtonian fluids has been made over a range of 12 orders of magnitude (10(-3) to 10(9) Pa s), extending from dilute aqueous solutions to the solid-like behaviour expected on approaching a glass transition. Using holographic optical tweezers to induce coalescence between two aerosol particles (volume ",

keywords = "HYGROSCOPICITY MODEL FRAMEWORK, SECONDARY ORGANIC AEROSOL, SUCROSE SOLUTIONS, GLASS-TRANSITION, SODIUM-CHLORIDE, PHASE-TRANSITIONS, AQUEOUS-SOLUTIONS, OPTICAL TWEEZERS, WATER, TEMPERATURE",

author = "Power, \{R. M.\} and Simpson, \{S. H.\} and Reid, \{J. P.\} and Hudson, \{A. J.\}",

year = "2013",

month = jun,

day = "1",

doi = "10.1039/c3sc50682g",

language = "English",

volume = "4",

pages = "2597--2604",

journal = "Chemical Science",

issn = "2041-6520",

publisher = "Royal Society of Chemistry",

number = "6",

}

TY - JOUR

T1 - The transition from liquid to solid-like behaviour in ultrahigh viscosity aerosol particles

AU - Power, R. M.

AU - Simpson, S. H.

AU - Reid, J. P.

AU - Hudson, A. J.

PY - 2013/6/1

Y1 - 2013/6/1

N2 - For the first time, a measurement of the viscosity of microparticles composed of Newtonian fluids has been made over a range of 12 orders of magnitude (10(-3) to 10(9) Pa s), extending from dilute aqueous solutions to the solid-like behaviour expected on approaching a glass transition. Using holographic optical tweezers to induce coalescence between two aerosol particles (volume

AB - For the first time, a measurement of the viscosity of microparticles composed of Newtonian fluids has been made over a range of 12 orders of magnitude (10(-3) to 10(9) Pa s), extending from dilute aqueous solutions to the solid-like behaviour expected on approaching a glass transition. Using holographic optical tweezers to induce coalescence between two aerosol particles (volume

KW - HYGROSCOPICITY MODEL FRAMEWORK

KW - SECONDARY ORGANIC AEROSOL

KW - SUCROSE SOLUTIONS

KW - GLASS-TRANSITION

KW - SODIUM-CHLORIDE

KW - PHASE-TRANSITIONS

KW - AQUEOUS-SOLUTIONS

KW - OPTICAL TWEEZERS

KW - WATER

KW - TEMPERATURE

UR - https://www.scopus.com/pages/publications/84877782854

U2 - 10.1039/c3sc50682g

DO - 10.1039/c3sc50682g

M3 - Article (Academic Journal)

SN - 2041-6520

VL - 4

SP - 2597

EP - 2604

JO - Chemical Science

JF - Chemical Science

IS - 6

ER -

The transition from liquid to solid-like behaviour in ultrahigh viscosity aerosol particles

Abstract

Research Groups and Themes

Keywords

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NEW STRATEGIES FOR SAMPLING, ANALYSING AND UNDERSTANDING AEROSOLS

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The transition from liquid to solid-like behaviour in ultrahigh viscosity aerosol particles

Abstract

Research Groups and Themes

Keywords

Access to Document

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NEW STRATEGIES FOR SAMPLING, ANALYSING AND UNDERSTANDING AEROSOLS

Cite this