Time Correlations in Fluid Transport Obtained by Sequential Rephasing Gradient Pulses

Siegfried Stapf*, Robin A. Damion, Ken J. Packer

*Corresponding author for this work

Research output: Contribution to journalArticle (Academic Journal)

21 Citations (Scopus)

Abstract

We present a basic experiment by which the evolution of the displacement probability density (propagator) of static or flowing fluid in N successive time intervals is obtained by single labeling, coupled with multiple rephasing events during the course of a pulsed field-gradient sequence. We term this type of sequence SERPENT: SEquential Rephasing by Pulsed field-gradients Encoding N Time-intervals. Realizations of the SERPENT experiment for the case N = 2 which include spin echo, stimulated echo, and Carr-Purcell pulse sequences are suggested. They have in common a spatial spin-labeling of the initial magnetization by a gradient of area q0, followed by successive rephasing via gradients q1 and q2 at times t = Δ1 and t = Δ2, respectively, where q0 + q1 + q2 = 0. A two-dimensional Fourier transform with respect to q1 and q2 gives directly the joint probability density W2(R1, Δ1; R2, Δ2) for displacements R1 and R2 in times Δ1 and Δ2, respectively. q1 and q2 may be in arbitrary directions. Assuming R1∥R2, the correlation coefficient ρR1,R2 then reflects the time-history of the fluctuating velocities. The behavior of the cross moment 〈R11) · R22)〉 can be obtained from either a full two-dimensional or a set of one-dimensional SERPENT measurements. Experimental results are presented for water flowing through a bed of packed glass beads. While Δ1 is appropriately chosen to sample the short-time velocity field within the system, increasing Δ2 clearly shows the loss of correlation when the average fluid element displacement exceeds the bead diameter.

Original languageEnglish
Pages (from-to)316-323
Number of pages8
JournalJournal of Magnetic Resonance
Volume137
Issue number2
DOIs
Publication statusPublished - 1999

Keywords

  • Flow
  • Multiple rephasing
  • Porous media
  • Time correlation
  • Two-dimensional propagators

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