Abstract
A number of recent transport and magnetization studies have shown signs of ferromagnetism in the LaAlO3/SrTiO3 heterostructure(1-6), an unexpected property with no bulk analogue in the constituent materials. However, no experiment thus far has provided direct information on the host of the magnetism(7-11). Here we report spectroscopic investigations of the magnetism using element-specific techniques, including X-ray magnetic circular dichroism and X-ray absorption spectroscopy, along with corresponding model calculations. We find direct evidence for in-plane ferromagnetic order at the interface, with Ti3+ character in the d(xy) orbital of the anisotropic t(2g) band. These findings establish a striking example of emergent phenomena at oxide interfaces.
Original language | English |
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Pages (from-to) | 703-706 |
Number of pages | 4 |
Journal | Nature Materials |
Volume | 12 |
Issue number | 8 |
Early online date | 2 Jun 2013 |
DOIs | |
Publication status | Published - Aug 2013 |
Keywords
- SUPERCONDUCTIVITY
- HETEROSTRUCTURES
- COEXISTENCE
- OXIDES