Unradiogenic lead in Earth's upper mantle

KW Burton, Benedicte Cenki-Tok, Fatima Mokadem, Jason Harvey, Abdelmouhcine Gannoun, Oliver Alard, Ian J Parkinson

Research output: Contribution to journalArticle (Academic Journal)peer-review

58 Citations (Scopus)


The mantle and continental crust—Earth’s main silicate reservoirs—have a lead isotope composition that is too radiogenic to have evolved from primitive Solar System material over 4.57 billion years1. To account for this imbalance, it has been suggested that unradiogenic lead may have partitioned into the metallic core2, 3, 4 or lower continental crust5. Alternatively, radiogenic lead could have been added to Earth later by meteorite impacts6. Unradiogenic lead was discovered in fragments of mantle rocks exhumed in the Horoman massif, Japan, implying that the mantle itself may provide a complementary reservoir of unradiogenic lead7. However, it is unclear why this unradiogenic component is not sampled by the melting that generates oceanic basalts8. Here we present double-spike lead isotope data for abyssal peridotite rocks, considered to represent suboceanic mantle, exposed on the Atlantic Ocean floor. We find that sulphides dated at about 1.83 billion years old and trapped as inclusions in silicate minerals preserve extremely unradiogenic lead isotope compositions. This unradiogenic lead could have been prevented from adding significantly to oceanic basalts if either the silicates shield the sulphide inclusions or if the sulphides reside in refractory mantle rocks that are rarely sampled during melting. We conclude that the lead isotope composition of the silicate Earth could be largely balanced by unradiogenic lead in sulphide in the mantle.
Original languageEnglish
Pages (from-to)570-573
Number of pages4
JournalNature Geoscience
Publication statusPublished - 22 Jul 2012


  • structural geology
  • Tectonics and Geodynamics
  • Geochemistry
  • Volcanology
  • Mineralogy
  • Petrology


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